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The Villalta Family Collection contains documents, clippings, and genealogical information about the Gaona family name and the Villalta family. This collection dates from 1624 to 1918. It is arranged into two series, Series I: Documents, 1678-1918 and Series II: Genealogy & Heraldry, 1624, in 21 folders in one box.

The Historical Documents Collection includes letters, deeds, bonds, receipts, orders, position appointments, writings, and other documents that are individual in nature and do not belong to any particular collection. The materials represent a number of prominent figures in the areas of art, literature, music, science, scholarship, business, law, military, politics, diplomacy, and religion. The items range in date from 1642-1977, but the bulk date from the 1760s through the 1920s. Most of the materials are American in origin, although some are from Mexico and Europe, particularly Great Britain.

Individuals represented in the collection include, but are not limited to:  Elizabeth Barrett Browning, Samuel Langhorne Clemens (Mark Twain), Charles Dickens, Oliver Wendell Holmes, Ralph Waldo Emerson, Washington Irving, Aldous Huxley, Rudyard Kipling, Ezra Pound, John Muir, Sigmund Freud, and Igor Stravinsky, Benjamin Butler, James Longstreet, Edmund Gaines Pendleton, Matthew Perry, William Tecumseh Sherman, Friedrich Wilhelm August Heinrich Ferdinand von Steuben, John Quincy Adams, Napoleon Bonaparte, Aaron Burr, Alexander Hamilton, Jefferson Davis, Ulysses Simpson Grant, Sam Houston, Andrew Jackson, James Madison, James Oglethorpe, William Howard Taft, Herbert Hoover, Thomas Paine, Woodrow Wilson, and King Louis XVIII.

The O. J. Tanner collection contains the following items: a scrapbook with various portraits of historical figures, a diary with notes on wills, an autograph scrapbook (including an autograph from President Ulysses Grant), a photostat copy of a letter by George Washington, an 1822 watercolor sketchbook, two photographs, a catalog and receipt from the Coral Gables Godspeed Bookshop, a 1743 pamphlet titled "Relation de la victorie Remporteé sur les Imperiaux, par les troupes du Roy, & celles du Roy de Serdaigne, dans la Bataille donneé prés de Guastalla, le 19 du mois dernier," and other pamphlets, clippings, programs, and prints.

The papers consist primarily of facsimilies and copies of documents relating to colonial Cuba.

The papers consist of correspondence including two letters of Tomás Estrada Palma, the first president of the Republic of Cuba and one letter of Generalísimo Máximo Gómez. The materials also include a photograph of the Shrine of Our Lady of Charity in El Cobre, Oriente and a photograph of "El Salto del Hanabanilla", which are placed with Cuban Photograph Collection, as well as, clippings, an album with drawings and poetry, Don Miguel Alberti's family tree, genealogy documents and the drawings of coats of arms.

The Finlay B. Matheson collection includes more than 2,411 photographs; 112 maps, surveys, and architectural plans; and 13 books related to William John Matheson and his immediate family. Estate documents and other documents containing historical and biographical information pertaining to the Matheson family and their various business ventures can also be found within this collection, as well as drawings, postcards, and some of the first aerial view photographs of Key Biscayne, Coconut Grove, the Miami River, and the Florida Keys. Florida's landscape during the early 20th century is captured throughout the various albums and scrapbooks and attests to a more leisurely lifestyle before the advent of skyscrapers and multi-lane highways. Furthermore, the collection provides an in-depth glimpse into the burgeoning social life of early inhabitants who gathered at the Biscayne Bay Yacht Club.

This collection features an array of scrapbooks, many of which are homemade, from the 19th and 20th centuries. Subjects covered in these scrapbooks include fashion, advertising, history, Robert Louis Stevenson, Pat Cannon's congressional run, garden clubs, cruises, and more. These scrapbooks are comprised of portraits, photographs, postcards, newspaper clippings, programs, brochures, maps, drawings, telegrams, and more. Some of the creators are unknowns or names without renown, but these scrapbooks highlight their personal tastes and interests, offering some unique insight into their lives.

The Thomas de Valcourt and Michael Lerner collection contains materials concerning 19th century New England poets and authors, most prominently Henry Wadsworth Longfellow, but also Henry David Thoreau, Washington Irving, Oliver Wendell Holmes, Ralph Waldo Emerson, Nathaniel Hawthorne, Walt Whitman, and minor figures. Much of the materials - which predominantly consists of prints, photographs, clippings, photocopies, newspapers, periodicals, postcards, reprints, poetry, and other formats - concerns their famous New England homes and their families' homes, and other literary landmarks in the vicinity. Most of the materials date from the late 19th and early 20th century.

Also included are a scrapbook of clippings of poetry, a 1962 plaster cast bust of Henry David Thoreau by Melvina Hoffman, an 1864 ceramic bust of Henry Wadsworth Longfellow by M. Milmore, two paperweights with depictions of the Longfellow house, a brick noted as "being used by Thoreau when adding to the family house on Virginia Road in Concord," and one copper ashtray.

The Elizabeth Wright collection predominantly contains materials relating to Richard Wagner and family members. The materials cover a wide range, including memorabilia, such as a Wagner-themed card game and a ceramic plaque of Richard Wagner, an original note by Siegfried Wagner and facsimiles of letters by Wagner, original photographs of Wagner family members as well as facsimiles and prints of Richard Wagner and others, original advertisements and programs of Wagner's operas, a radio transcript and a typescript about Wagner's composition and staging, and a series of prints depicting scenes from Wagner's operas.

There are also several items not related to Wagner. These are a letter from W. Somerset Maugham, an autographed print of mezzo-soprano Mariana Paunova, and prints of other composers such as Beethoven, Mozart, Liszt, and Richter.

The papers document activities of J. M. Portuondo in capacity of a professor of Internal Medicine at the University of Havana, a writer and a faculty member of the University of Miami School of Medicine.  The materials include books, pamphlets, periodicals, clippings, circular letters, typescripts of anti-communist writings by Portuondo, reports, a poem by Portuondo, speeches by him, copies of his medical diplomas, a historical map of Havana, and photostats of a photograph and of a letter from José Martí to José Portuondo.

The Alan Crockwell Collection contains a variety of materials from different sources that document the history of Miami, Coconut Grove, Coral Gables, and greater Miami-Dade County. Much of the content is related to Ralph Middleton Munroe and his family. Topically, the papers also address criminal history in Miami-Dade County, historic buildings in Coconut Grove including the Barnacle and the Coconut Grove Library, the history of the University of Miami, and the early settling of Miami-Dade County. The dates of items range from 1873 into the 1970s.

The collection documents Georgina Shelton's involvement in Lyceum and Lawn Tennis Club, Havana, Cuba are the most important ones in this collection. Materials also include articles about and by Hilda Perera, postcards of Mexico from 1920, programs from John J. Koubek Memorial Center, clippings, correspondence and newspaper from 1876.

Research material from noted author and historian, Arva Moore Parks McCabe (1939-2020). Born in Miami, Florida, Arva had written countless books on Florida's eclectic history, including The Forgotten Frontier: Florida through the Lens of Ralph Middleton Munroe, Miami, the Magic City, and George Merrick, Son of the South Wind: Visionary Creator of Coral Gables. She also served as chief curator, interim director, and chair of the Coral Gables Museum.

This collection focuses heavily on George E. Merrick, Coral Gables, and other research topics used in her writings. It also features a large assortment of archival material: booklets, books, magazines, posters, photographs, negatives, pamphlets, postcards, maps, ephemera, newspapers, and guides about Miami and other notable cities and famous people related to South Florida.

This collection contains correspondence from the Barnott family, primarily letters to and from Mary A. Barnott, the wife of Edward Barnott. The two of them were early settlers of the Biscayne Bay area in the 1870s, and the family's letters document much of the day-to-day affairs of life in Miami at the turn of the 20th century. They were also close friends with William H. Gleason, the founder of the Biscayne community, and his family, all of whose correspondence with the Barnotts can be found in this collection. Furthermore, the collection contains other archival materials, such as clippings, notes, old checks, and advertisements.

The papers include letters from various prominent Cuban figures; among them Tomás Estrada Palma, Salvador Cisneros, Lola R. de Tió, Armando Menocal, Mario Menocal and others.  The materials also consist of newspaper clippings about sugar industry and some photographs.

The Charles T. Simpson collection contains photographs, account statements, letters, minutes, contracts, typescripts, articles, certificates, membership cards, manuscripts, notes, photocopies, and a plant specimen, which document the lengthy botanical and zoological career of the early 20th century naturalist.