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The Historical Documents Collection includes letters, deeds, bonds, receipts, orders, position appointments, writings, and other documents that are individual in nature and do not belong to any particular collection. The materials represent a number of prominent figures in the areas of art, literature, music, science, scholarship, business, law, military, politics, diplomacy, and religion. The items range in date from 1642-1977, but the bulk date from the 1760s through the 1920s. Most of the materials are American in origin, although some are from Mexico and Europe, particularly Great Britain.

Individuals represented in the collection include, but are not limited to:  Elizabeth Barrett Browning, Samuel Langhorne Clemens (Mark Twain), Charles Dickens, Oliver Wendell Holmes, Ralph Waldo Emerson, Washington Irving, Aldous Huxley, Rudyard Kipling, Ezra Pound, John Muir, Sigmund Freud, and Igor Stravinsky, Benjamin Butler, James Longstreet, Edmund Gaines Pendleton, Matthew Perry, William Tecumseh Sherman, Friedrich Wilhelm August Heinrich Ferdinand von Steuben, John Quincy Adams, Napoleon Bonaparte, Aaron Burr, Alexander Hamilton, Jefferson Davis, Ulysses Simpson Grant, Sam Houston, Andrew Jackson, James Madison, James Oglethorpe, William Howard Taft, Herbert Hoover, Thomas Paine, Woodrow Wilson, and King Louis XVIII.

The Jamaica Manuscripts Collection contains 20 documents, most of which concern Jamaica in a variety of ways (others are regarding the British West Indies at large). Included, among other things, are plantation records, correspondence, journals, official documents such as power of attorney documents and affidavits, notes on the climate of Jamaica, and Spanish reports on English possessions.  Some of these are originals, where others are later 20th century documents about Jamaica or typescripts of letters.

The papers consist of correspondence including two letters of Tomás Estrada Palma, the first president of the Republic of Cuba and one letter of Generalísimo Máximo Gómez. The materials also include a photograph of the Shrine of Our Lady of Charity in El Cobre, Oriente and a photograph of "El Salto del Hanabanilla", which are placed with Cuban Photograph Collection, as well as, clippings, an album with drawings and poetry, Don Miguel Alberti's family tree, genealogy documents and the drawings of coats of arms.

The Theodore Bolton Papers contains materials that span from across the entirety of Bolton's life. Bolton was active as a book illustrator and as an art historian, and so there are typescripts, manuscripts, reprints, and periodicals, as well as sketches, prints, drawings, engravings, and sketchbooks.

Bolton's sketches are primarily illustrations for books or Christmas Card designs. Also among the sketches are several done by other illustrators. These include an original illustration by Timothy Cole, as well as a number of original sketches by James Daugherty. Many of these sketches are on Christmas cards sent to Theodore Bolton and Helen, his wife.

Beside his manuscripts and illustrations, of special notice are travel journals by Bolton spanning across several decades, each of which contain illustrations of the places that he visited, and 20 Confederate States of America Banknotes.

The Thomas de Valcourt and Michael Lerner collection contains materials concerning 19th century New England poets and authors, most prominently Henry Wadsworth Longfellow, but also Henry David Thoreau, Washington Irving, Oliver Wendell Holmes, Ralph Waldo Emerson, Nathaniel Hawthorne, Walt Whitman, and minor figures. Much of the materials - which predominantly consists of prints, photographs, clippings, photocopies, newspapers, periodicals, postcards, reprints, poetry, and other formats - concerns their famous New England homes and their families' homes, and other literary landmarks in the vicinity. Most of the materials date from the late 19th and early 20th century.

Also included are a scrapbook of clippings of poetry, a 1962 plaster cast bust of Henry David Thoreau by Melvina Hoffman, an 1864 ceramic bust of Henry Wadsworth Longfellow by M. Milmore, two paperweights with depictions of the Longfellow house, a brick noted as "being used by Thoreau when adding to the family house on Virginia Road in Concord," and one copper ashtray.

The Elizabeth Wright collection predominantly contains materials relating to Richard Wagner and family members. The materials cover a wide range, including memorabilia, such as a Wagner-themed card game and a ceramic plaque of Richard Wagner, an original note by Siegfried Wagner and facsimiles of letters by Wagner, original photographs of Wagner family members as well as facsimiles and prints of Richard Wagner and others, original advertisements and programs of Wagner's operas, a radio transcript and a typescript about Wagner's composition and staging, and a series of prints depicting scenes from Wagner's operas.

There are also several items not related to Wagner. These are a letter from W. Somerset Maugham, an autographed print of mezzo-soprano Mariana Paunova, and prints of other composers such as Beethoven, Mozart, Liszt, and Richter.

The papers document activities of J. M. Portuondo in capacity of a professor of Internal Medicine at the University of Havana, a writer and a faculty member of the University of Miami School of Medicine.  The materials include books, pamphlets, periodicals, clippings, circular letters, typescripts of anti-communist writings by Portuondo, reports, a poem by Portuondo, speeches by him, copies of his medical diplomas, a historical map of Havana, and photostats of a photograph and of a letter from José Martí to José Portuondo.

The Charles T. Simpson collection contains photographs, account statements, letters, minutes, contracts, typescripts, articles, certificates, membership cards, manuscripts, notes, photocopies, and a plant specimen, which document the lengthy botanical and zoological career of the early 20th century naturalist.

This collection contains typescripts, photocopies and photographs regarding the history of the confederate submarine H. L. Hunley.

The Papers consist primarily of  typescripts, correspondence, photographs, diaries, scrapbooks, clippings and other primary source materials documenting the life and career of Marjory Stoneman Douglas.

George Augustus Moore (1852–1933) was an Irish novelist, short-story writer, poet, art critic, memoirist and dramatist.

The George Moore Collection contains correspondence, an undated manuscript titled "Scenario," the galley proofs with corrections for his 1885 novel Mummer's Wife, and a typescript for his 1894 novel Esther Waters.

The correspondence consists of a series of letters and telegraphs between Moore and New York playwright and writer Edward Knoblauch (1874-1945), a letter from Moore to a "Nachey," several letters without a recipient name, two letters from D. M. Beth at Riverside Press Unlimited, a book printer from Edinburgh, discussing corrections on Moore's 1921 novel Heloise and Abelard.

Charles Arnould Hentz (1827-1894) was a physician practicing in the rural South in the years leading up to and through the Civil War. Dr. Hentz is famously known for his diary that he kept for more than twenty years, which depicts the demanding work of a physician in an age before medicine could reliably cure patients. The collection contains a two-volume carbon typescript of his autobiography that he penned at the end of his life. Also included is a pamphlet titled "Le Conventionnel Hentz Depute de la Moselle," translated into English, about Nicolas Hentz, a député of the Moselle to the French National Convention.

This collection consists of an undated, unpublished typescript by Clark Daniel Stearns, U.S. Naval Officer and former Governor of the American Samoa. The typescript is titled "American Samoa."